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RAS Chemistry & Material ScienceКоординационная химия Russian Journal of Coordination Chemistry

  • ISSN (Print) 0132-344X
  • ISSN (Online) 3034-5499

Donor–acceptor chromophores based on coordination polymers of silicon(IV) and germanium(IV)

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PII
S3034549925030025-1
DOI
10.7868/S3034549925030025
Publication type
Article
Status
Published
Authors
K. V. Arsenyeva
  • Affiliation: Razuvaev Institute of Organometallic Chemistry, Russian Academy of Sciences
Volume/ Edition
Volume 51 / Issue number 3
Pages
165-175
Abstract
New charge-transfer complexes with pyrazine are synthesized from germanium(IV) and silicon(IV) bis(catecholates): 36Сat2Ge, 35Cat2Ge, and 36Сat2Si (36Сat and 35Cat are 3,6- and 3,5-di-tert-butylpyrocatechol dianions, respectively). The synthesized compounds in the crystalline state are 1D coordination polymers with the octahedral environment of the complexing agent. The electronic absorption spectra of suspensions of the crystalline compounds in Nujol demonstrate an absorption in a range of 450–800 nm causing their intense color. A set of the spectral and theoretical studies indicates that the synthesized metal-organic frameworks of silicon and germanium can be considered as donor–acceptor chromophores with the photoinduced interligand charge transfer between the donor catecholate and acceptor pyrazine ligands.
Keywords
кремний германий редокс-активные лиганды координационные полимеры комплекс с переносом заряда
Date of publication
17.03.2025
Year of publication
2025
Number of purchasers
0
Views
50

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